Measurements of Aerosol Parameters
Aboard
the DC-8
during the Transport and Chemical Evolution over the Pacific Mission
Chemistry
and Dynamics Branch We will
provide in situ measurements of aerosol size distribution, volatility, and
optical characteristics aboard the NASA DC-8 during the Transport and Chemical
Evolution over the Pacific (TRACE-P) mission.
The instrument suite will include: 1) an ultrafine
condensation nuclei counter (CNC) to determine the number of particles
between 0.003 and 0.012 mm (ultrafine CN)
2) a pair of standard CNCs, one with a heated inlet, to measure the number and
volatility of aerosols > 0.012 mm; 2)
a scanning mobility particle spectrometer (SMPS) coupled to a CNC to obtain
90-second resolution size distributions for 0.010 to 0.250 mm
diameter particles; 3) A PMS passive cavity aerosol spectrometer probe (PCASP)
for obtaining dry particle size distributions over the 0.1 to 3.0 mm
size-diameter range; 4) A PMS forward scattering spectrometer probe (FSSP-300)
to determine particle size distributions over the 0.35 to 3.0 mm
size-diameter range 5) a 3-wavelength integrating nephelometer for measuring
wavelength-dependent aerosol scattering; 6) an aethelometer for determining
total aerosol (i.e., black carbon) absorption; and 7) a cloud, aerosol, and
precipitation spectrometer (CAPS) to provide improved particle size information
over the 0.3 to 1550 mm
size range along with particle asphericity and cloud liquid water
content. The parameters that
will be archived are listed in Table 1 below.
The PCASP, FSSP, and CAPS are designed for aircraft use and will be
mounted in the existing aerosol canisters that attach to the DC-8 wingtips.
The FSSP-300 and CAPS have open sample cavities and thus avoid many of
the problems associated with anisokinetic sampling that are particularly serious
for super micron-sized aerosols. The
PCASP has an enclosed sample cavity into which samples are drawn through a short
(about 4 cm) length of heated capillary tubing.
Our calculations suggest that, because the probe is used to size fine
aerosols that are much less sensitive to inertial and gravitational effects,
this sample extraction technique minimally disturbs the size and number density
of the ambient aerosol. All
probes will be calibrated prior to the missions using aerosols of known
refractive index and size. The CNCs,
SMPS, nephelometer, and aethelometer are mounted within the aircraft cabin. Sample air for these instruments will be drawn in through two
window-mounted inlets: a scoop-type inlet that shunts particles larger the ~1 mm
and an isokinetic, forward-facing inlet that efficiently transmits coarse
aerosols. The scoop inlet has been
installed onboard the DC-8 for several previous missions and will deliver
samples to the CNCs and SMPS systems. Its
design minimizes problems with precipitation particle shattering which permits
collecting interstitial samples within clouds.
Sample air enters though this probe, passes in front of a small sample
extraction orifice located within a manifold mounted on the side of the rack,
and is subsequently dumped overboard through a rear-facing tube mounted on the
aircraft window plate. Air
withdrawn though the sample orifice is diluted with a concentric flow of
filtered air to maintain the sensor systems at a constant pressure of 160 Torr
regardless of aircraft altitude. Table 1. List of
parameters to be archived. Resolution Limit
of Parameter Units seconds Precision Detection Total
aerosols > 0.004 um cm-3 1 20% 10 Total
aerosols > 0.012 um " 1 10% 1 Nonvolatile
aerosols > 0.012 um " 1 10% 1 Mean
Nucleation Mode Diameter (0.01
to 0.1 mm) mm 90 .01 mm - Nucleation
Mode Number Density cm-3 90 20% 10 Nucleation
Mode Surface Area cm-3 90 50% - Mean
Accumulation Mode Diameter (0.1
to 1.0 mm) mm 1 .05 mm - Accumulation
Mode Number Density cm-3 1 20% 1 Accumulation
Mode Surface Area mm -2 cm-3 1 50% - Mean
Coarse Mode Diameter (1.0 to 20
mm ) mm 1 0.2
mm Coarse
Mode Number Density cm-3 1 20% 0.1 Coarse
Mode Surface Area mm -2 cm-3 1 50% - Mean
Precipitation Mode Diameter (0.05
to 1.6 mm) cm 1 20% 0.1 Precipation
Mode Number Density m-3 1 20% 10 Precipitation
Mode Surface Area mm-2
m-3 1 50% - Precipitation
Mode Volume (calculated) mm-3
m-3 1 50% - Liquid
Water Content g
m-3 1 20% 0.01 Total
Aerosol Surface Area (0.01 to 1.6 mm) mm-2
cm-3 90 50% Total
Aerosol Volume mm-3
cm-3 Aerosol
Phase (Ice or Water) - 1 - - Accumulation
Mode Refractive Index - 1 5% - Aerosol
Scattering Coefficient (450 nm) m-1 1 1.00E-07 Aerosol
Scattering Coefficient (550 nm) m-1 1 1.00E-07 Aerosol
Scattering Coefficient (700 nm) m-1 1 1.00E-07 Black
Carbon mg
m-3 60 10% 0.1
Wesley R. Cofer, III, Co-Investigator
Edward L. Winstead, Co-Investigator
Atmospheric
Sciences Competency
NASA
Langley Research Center